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Rickertsen, Dillon R.; Ma, Longle; Paul, Anirudra; Abboud, Khalil A.; Seidel, Daniel (, SynOpen)null (Ed.)Abstract Amines such as 1,2,3,4-tetrahydroisoquinoline undergo redox-neutral annulations with ortho-(nitromethyl)benzaldehyde. Benzoic acid acts as a promoter in these reactions, which involve concurrent amine α-C–H bond and N–H bond functionalization. Subsequent removal of the nitro group provides access to tetrahydroprotoberberines not accessible via typical redox-annulations. Also reported are decarboxylative annulations of ortho-(nitromethyl)benzaldehyde with proline and pipecolic acid.more » « less
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Chen, Weijie; Paul, Anirudra; Abboud, Khalil A.; Seidel, Daniel (, Nature Chemistry)null (Ed.)
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Lin, Yingfu; Hirschi, William J.; Kunadia, Anuj; Paul, Anirudra; Ghiviriga, Ion; Abboud, Khalil A.; Karugu, Rachael W.; Vetticatt, Mathew J.; Hirschi, Jennifer S.; Seidel, Daniel (, Journal of the American Chemical Society)
